The brain will entrain to the strongest stimulus. If you combine binaural beats with isochronic tones, your brainwaves will entrain to the isochronic tones. If anything, when you combine the two I believe it makes the track less effective because it makes it harder for the brain to decipher between the two and synchronise to a single beat. There are lots of websites with compelling marketing about the benefits of combining the two together in some funky way, but I haven’t seen any research or lots of anecdotal feedback even to suggest it’s effective to combine them.
Again, it is important to be cautious of claims for things like these, and to find a brainwave entrainment seller that you can trust to make quality audios. It is incredibly easy for someone to throw together an audio without much to it and make all kinds of claims about what it can do for you. Please feel free to read through our reviews on the site to see some of the products I have tested and found to be of a reputable quality.
With brainwave entrainment audio, the brain will "catch on" and follow (entrain to) the desired brainwave frequency. BrainAscend uses the binaural and isochronic type of entrainment together with amplitude modulation. Isochronic tones have been proven to be the most effective brainwave entrainment technology and does not require headphones.  Binaural beats are powerful when it comes to increasing synchronization of the brain hemispheres. You don't have to use headphones, though it is suggested. This is automatic meditation. Press play, close your eyes and BrainAscend does the rest!
I can offer a hypothetical--however do not know know practical it will turn out to be. There is a fair amonut of bad science on this topic on you tube. The gamma wave frequency is associated with attentional focus and arguably a unified sense of self. If it could be entrained it should lead to a meditative focus-like exceptionally well-trained meditators. Some but not all studies on meditating Buddhist monks suggest this is so. Does this really and more generally occur--I will say there is nothing lost in trying--we all go into a 40Hz range on occasion without ill effect-- but I would not put confidence in the purported methods out there at present. Good luck.
Applying brainwave entrainment in the alpha range may result in benefits similarly found with Zen or Transcendental Meditation. These benefits extend throughout the body and include improved breathing patterns, higher physical energy levels, an improved outlook, increased sports performance, improved relationships, and increased workplace satisfaction and performance … just to name a few.

“…humans have always been intrigued by the possibilities for influencing mental functioning that emerge from combining rhythmic sound and rhythmic light stimulation. Ancient rituals for entering trance states often involved both rhythmic sounds in the form of drum beats, clapping, or chanting and flickering lights produced by candles, torches, bonfires, or long lines of human bodies passing before the fire and chopping the light into mesmerizing rhythmic flashes. From Greek plays to Western opera, our most popular entertainment forms have made use of combinations of lights and sounds. Some composers, such as the visionary Scriabin, actually created music intended to be experienced in combination with rhythmic light displays.”
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Memory: There is not sufficient evidence to suggest that brainwave entrainment improves memory. However since cognitive function improves as a result of entrainment, short and/or long term memory may be improved by stimulation with certain frequencies. While lower frequencies may be beneficial for recalling certain memories, conscious processing of the memories generally requires sufficient beta.
A study by Tina Huang, PhD, and Christine Charyton, published in the September 2008 issue of the journal, Alternative Therapies examined the results of twenty previous studies measuring the effectiveness of brainwave entrainment for improvements in cognitive dysfunction and deficits, stress reduction, pain management, migraine and headache control, pre-menstrual syndrome, and behavioral difficulties, and all showed significant improvement in symptoms using entrainment techniques.

There appeared to be some evidence that 10 Hz stimulation (alpha waves) improved anxiety, but it wasn’t statistically significant. A study that utilized a ramping format of alpha to theta to delta waves (over the course of 10 minutes) found a significant improvement in anxiety. In terms of long-term stress, there is evidence that alpha and beta stimulation improved measures of “competence” and “emotional exhaustion.”
Miscellaneous reports have also been made about the advantages of brainwave entrainment with the reviews of numerous users stating that the it can assist in increasing sex drive. Research shows that relaxation, meditation, and good self esteem ensures normal body functions. Furthermore, the brainwave entertainment allows your body to flow in rhythm with the beats therefore if your brain accepts and blends with certain frequencies, this could account for the enhanced sex drive.
Brainwave entrainment is a colloquialism for such 'neural entrainment', which is a term used to denote the way in which the aggregate frequency of oscillations produced by the synchronous electrical activity in ensembles of cortical neurons can adjust to synchronize with the periodic vibration of an external stimuli, such as a sustained acoustic frequency perceived as pitch, a regularly repeating pattern of intermittent sounds, perceived as rhythm, or of a regularly rhythmically intermittent flashing light.
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